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The most common way to block a sender is through the AOL Mail website on a computer. to your AOL Mail account. Open the email from the sender you want to block.

Warning: This will prevent any new person from emailing you unless you add their email address to your AOL Contacts first. How to Unblock an Email Address

While the mobile app (available on iOS and Android) does not always have a dedicated "Block" button in the settings, you can achieve the same result by using the "Spam" feature.